Edited by Marlan O. Scully, Texas A&M University, College Station, TX, and approved October 19, 2020 (received for review May 27, 2020)
Author contributions: N.J.C. designed research; and N.J.C. and M.G.J. performed research, derived the formulas, discussed the results, and wrote the paper.
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We uncover an unsuspected quantum interference mechanism, which originates from the indistinguishability of identical bosons in time. Specifically, we build on the Hong–Ou–Mandel effect, namely the “bunching” of identical bosons at the output of a half-transparent beam splitter resulting from the symmetry of the wave function. We establish that this effect turns, under partial time reversal, into an interference effect in a quantum amplifier that we ascribe to time-like indistinguishability (bosons from the past and future cannot be distinguished). This hitherto unknown effect is a genuine manifestation of quantum physics and may be observed whenever two identical bosons participate in Bogoliubov transformations, which play a role in many facets of physics.
The celebrated Hong–Ou–Mandel effect is the paradigm of two-particle quantum interference. It has its roots in the symmetry of identical quantum particles, as dictated by the Pauli principle. Two identical bosons impinging on a beam splitter (of transmittance 1/2) cannot be detected in coincidence at both output ports, as confirmed in numerous experiments with light or even matter. Here, we establish that partial time reversal transforms the beam splitter linear coupling into amplification. We infer from this duality the existence of an unsuspected two-boson interferometric effect in a quantum amplifier (of gain 2) and identify the underlying mechanism as time-like indistinguishability. This fundamental mechanism is generic to any bosonic Bogoliubov transformation, so we anticipate wide implications in quantum physics.
The laws of quantum physics govern the behavior of identical particles via the symmetry of the wave function, as dictated by the Pauli principle (1). In particular, it has been known since Bose and Einstein (2) that the symmetry of the bosonic wave function favors the so-called bunching of identical bosons. A striking demonstration of bosonic statistics for a pair of identical bosons was achieved in 1987 in a seminal experiment by Hong, Ou, and Mandel (HOM) (3), who observed the cancellation of coincident detections behind a 50:50 beam splitter (BS) when two indistinguishable photons impinge on its two input ports (Fig. 1A). This HOM effect follows from the destructive two-photon interference between the probability amplitudes for double transmission and double reflection at the BS (Fig. 1B). Together with the Hanbury Brown and Twiss effect (4, 5) and the violation of Bell inequalities (6, 7), it is often viewed as the most prominent genuinely quantum feature: it highlights the singularity of two-particle quantum interference as it cannot be understood in terms of classical wave interference (8, 9). It has been verified in numerous experiments over the last 30 y (see, e.g., refs. 101112–13), even in case the single photons are simultaneously emitted by two independent sources (1415–16) or within a silicon photonic chip (17, 18). Remarkably, it has even been experimentally observed with He metastable atoms, demonstrating that this two-boson mechanism encompasses both light and matter (19).


(A) If two indistinguishable photons (represented in red and green for the sake of argument) simultaneously enter the two input ports of a 50:50 BS, they always exit the same output port together (no coincident detection can be observed). (B) The probability amplitudes for double transmission (Left) and double reflection (Right) precisely cancel each other when the transmittance is equal to 1/2. This is a genuinely quantum effect, which cannot be described as a classical wave interference. (C) The correlation function exhibits an HOM dip when the time difference
Here, we explore how two-boson quantum interference transforms under reversal of the arrow of time in one of the two bosonic modes (Fig. 2A). This operation, which we dub partial time reversal (PTR), is unphysical but nevertheless central as it allows us to exhibit a duality between the linear optical coupling effected by a BS and the nonlinear optical (Bogoliubov) transformation effected by a parametric amplifier. As a striking implication of these considerations, we predict a two-photon interferometric effect in a parametric amplifier of gain 2 (which is dual to a BS of transmittance 1/2). We argue that this unsuspected effect originates from the indistinguishability between photons from the past and future, which we coin “time-like” indistinguishability as it is the partial time-reversed version of the usual “space-like” indistinguishability that is at work in the HOM effect.


(A) BS under PTR, flipping the arrow of time in mode
Since Bogoliubov transformations are ubiquitous in quantum physics, it is expected that this two-boson interference effect in time could serve as a test bed for a wide range of bosonic transformations. Furthermore, from a deeper viewpoint, it would be fascinating to demonstrate the consequence of time-like indistinguishability in a photonic or atomic platform as it would help in elucidating some heretofore overlooked fundamental property of identical quantum particles.
Hong–Ou–Mandel Effect
The HOM effect is a landmark in quantum optics as it is the most spectacular manifestation of boson bunching. It is a two-photon intrinsically quantum interference effect where the probability amplitude of both photons being transmitted cancels out the probability amplitude of both photons being reflected. A 50:50 BS effects the single-photon transformations (for details, see Materials and Methods, Gaussian Unitaries for a BS and PDC)
Partial Time Reversal
Bogoliubov transformations on two bosonic modes comprise passive and active transformations. The BS is the fundamental passive transformation, while parametric down conversion (PDC) gives rise to the class of active transformations (also called nondegenerate parametric amplification). Although the involved physics is quite different (a simple piece of glass makes a BS, while an optically pumped nonlinear crystal is needed to effect PDC), the Hamiltonians generating these two unitaries are amazingly close, namely
The underlying concept of PTR will be formalized in Eq. 7, but we first illustrate this duality between a BS and PDC with the simple example of Fig. 2A, where
These examples reflect the existence of a general duality between a BS and PDC. Indeed, as demonstrated in Materials and Methods, Proof of PTR Duality, partial transposition in Fock basis gives rise to PTR duality
The notion of time reversal can be conveniently interpreted using the so-called “retrodictive” picture of quantum mechanics (21). Along this line, PTR must be understood here as the fact that the “retrodicted” state of mode
Two-Boson Interference in an Amplifier
Due to this duality, the HOM effect for a BS of transmittance 1/2 immediately suggests the possible existence of a related interferometric suppression effect in a PDC of gain 2, namely


(A) Probability
The dependence of the probability of detecting a single pair (
Space-Like vs. Time-Like Indistinguishability
The origin of the two-boson quantum interference effect that we predict can be traced back to boson indistinguishability, similarly as for the HOM effect albeit in a time-like version (involving bosons from the past and future). We first recall that the HOM effect originates from what can be viewed as space-like indistinguishability (Fig. 4, Upper). When two photons impinge on a BS of transmittance


The HOM effect (Upper) is due to space-like indistinguishability: the double-transmission path (of amplitude
We now argue that it is the exchange of indistinguishable photons in time that is responsible for the interference effect in an amplifier (Fig. 4, Lower). When two photons impinge on a PDC with gain
Discussion and Conclusion
The role of time reversal in quantum physics has long been a fascinating subject of questioning (see, e.g., ref. 22 and references therein), but the key idea of the present work is to consider a bipartite quantum system (two bosonic modes) with counterpropagating times. Incidentally, we note that the notion of time reversal has been exploited in the context of defining separability criteria (23, 24), but this seems to be unrelated to PTR duality. Further, the link between time reversal and optical-phase conjugation has been mentioned in the quantum optics literature (see, e.g., ref. 25), but it exploits the fact that the complex conjugate of an electromagnetic wave is the time-reversed solution of the wave equation (the phase conjugation time-reversal mirror concerns one mode only). The PTR duality introduced here bears some resemblance with an early model of lasers (26) based on the coupling of an “inverted” harmonic oscillator (having a negative frequency
In this work, we have promoted PTR as the proper way to approach the duality between passive and active bosonic transformations. As a compelling application of PTR duality, we have unveiled a hitherto unknown quantum interference effect, which is a manifestation of quantum indistinguishability for identical bosons in active transformations (space-like indistinguishability, which is at the root of the HOM effect, transforms under PTR into time-like indistinguishability). The interferometric suppression of the coincident
The experimental verification of this effect can be envisioned with present technologies (see Experimental Scheme). A coincidence probability lower than 25% would be sufficient to rule out a classical interpretation, which could in principle be reached with a moderate gain of 1.28 (see Classical Baseline). Observing time-like two-photon interference in experiments involving active optical components would then be a highly valuable metrology tool given that the HOM dip is commonly used today as a method to benchmark the reliability of single-particle sources and mode matching. More generally, the interference of many photons scattered over many modes in a linear optical network has generated a tremendous interest in the recent years, given the connection with the “boson sampling” problem [i.e., the hardness of computing the permanent of a random matrix (29)], and technological progress in integrated optics now makes it possible to access large optical circuits (see, e.g., ref. 30). In this context, it would be exciting to uncover new consequences of PTR duality and time-like interference.
Finally, we emphasize that our analysis encompasses all bosonic Bogoliubov transformations, which are widespread in physics, appearing in quantum optics, quantum field theory, or solid-state physics, but also in black hole physics or even in the Unruh effect (describing an accelerating reference frame). This suggests that time-like quantum interference may occur in various physical situations where identical bosons participate in such a transformation. Beyond bosons, let us point out an intriguing connection with the notion of “crossing” in quantum electrodynamics (31, 32). Crossing symmetry refers to a substitution rule connecting two scattering matrix elements that are related by a Wick rotation (antiparticles being turned into particles going backward in time). For example, the scattering of a photon by an electron (Compton scattering) and the creation of an electron–positron pair by two photons are processes that are related to each other by such a substitution rule (see, e.g., ref. 33). This is in many senses analogous to the PTR duality described here: since a photon (or truly neutral boson) is its own antiparticle, we may view PTR duality as a substitution rule connecting the BS diagram to the PDC diagram. We hope that this connection with quantum electrodynamics may open up even broader perspectives.
Materials and Methods
Gaussian Unitaries for a BS and PDC.
Passive and active Gaussian unitaries are effected by linear optical interferometry or parametric amplification, respectively (34). The fundamental passive two-mode Gaussian unitary, namely the BS unitary
The action of
Example of PTR.
We illustrate the PTR duality between a BS and PDC by considering the additional example of a BS with


(A) PTR duality in a more general case with
Proof of PTR Duality.
The PTR duality is illustrated in Table 1 for few photons. As expressed by Eq. 7, it can be viewed as a consequence of partial transposition of the state of mode

| BS | PDC |
The second column (PDC) is obtained from the first column (BS) by timereversing mode


(A) General statement of the PTR duality as expressed in Eq. 7, when
We now prove PTR duality by reexpressing Eq. 24 in the Heisenberg picture, namely
Similar equations can be derived starting from
Note that PTR duality can be reexpressed by using the identity
Retrodictive Picture of Quantum Mechanics.
In the usual, predictive approach of quantum mechanics, one deals with the preparation of a quantum system followed by its time evolution and ultimately, its measurement. Specifically, one uses the prior knowledge on the state


(A) Predictive (Left) and retrodictive (Right) pictures, describing the same experiment where state
The retrodictive picture can be successfully exploited in different situations [for example, to characterize the quantum properties of an optical measurement device (35)], but it is always used in lieu of the predictive picture. Here, we instead combine it with the predictive picture in order to properly define PTR duality and describe a composite system that is propagated partly forward and partly backward in time, as represented in Fig. 7 B, Right. Specifically, we consider a composite system prepared in a product state
In our analysis of a BS under PTR, we have
Two-Photon Interference in a BS and PDC.
The HOM effect can be simply understood by calculating the probability amplitude for coincident detection
Now, we examine the corresponding quantum interferometric suppression in a PDC and its dependence in the parametric gain
Extension to a PDC with Integer Gain.
We may also consider the case where the gain takes a larger integer value (e.g.,


Extended quantum interferometric suppression in an amplifier where the detection of
Experimental Scheme.
The HOM effect is considered a most spectacular evidence of genuinely quantum two-boson interference, and we expect the same for its PTR counterpart as it admits no classical interpretation. The experimental verification of our effect can be envisioned with present technologies, as sketched in Fig. 9. We would need two single-photon sources, which could be heralded by the detection of a trigger photon at the output of a PDC with low gain (the single photon being prepared conditionally on the detection of the trigger photon in the twin beam). The two single photons would impinge on a PDC of gain 2, whose output modes should be monitored: the probability of detecting exactly one photon on each mode should be suppressed as a consequence of time-like indistinguishability. In principle, photon number resolution would be needed in order to discriminate the output term with one photon pair (

![Schematic of a potential demonstration of two-photon quantum interference in the amplification of light with gain 2. Two heralded single-photon sources (exploiting an avalanche photodetector [APD]) are used to feed the signal and idler modes of a PDC, and two photon number-resolving (PNR) detectors are used to monitor the presence of a single photon in each output port. The two-photon interference effect would be demonstrated by measuring a depletion of fourfold coincidences between the two trigger photons (heralding the preparation of two single photons) and the two output photons (here, the detectors should filter out the output states with ≥2 photons on each mode). The dominant terms will then consist of the stimulated annihilation of the two input photons (witnessed by two trigger photons but no output photons) as well as the stimulated emission of a photon pair (witnessed by two output photons but no trigger photons). When the time lapse between the detection of the trigger and output photons is close to zero (which means a perfect match of the timing of the output photons originating from the input photons associated with the trigger photons) the two terms should interfere destructively.](/dataresources/secured/content-1765760018179-aadf3d74-d338-4ace-9ff8-6de8b4593915/assets/pnas.2010827117fig09.jpg)
Schematic of a potential demonstration of two-photon quantum interference in the amplification of light with gain 2. Two heralded single-photon sources (exploiting an avalanche photodetector [APD]) are used to feed the signal and idler modes of a PDC, and two photon number-resolving (PNR) detectors are used to monitor the presence of a single photon in each output port. The two-photon interference effect would be demonstrated by measuring a depletion of fourfold coincidences between the two trigger photons (heralding the preparation of two single photons) and the two output photons (here, the detectors should filter out the output states with
Demonstrating this effect would be invaluable in view of the fact that the HOM dip is widely used to test the indistinguishability of single photons and to benchmark mode matching: it witnesses the fact that the photons are truly indistinguishable (they admit the same polarization and couple to the same spatiotemporal mode). For example, HOM experiments have been used to test the indistinguishability of single photons emitted by a semiconductor quantum dot in a microcavity (10), while the interference of two single photons emitted by two independently trapped rubidium-87 atoms has been used as an evidence of their indistinguishability (15). The HOM effect has also been generalized to three-photon interference in a three-mode optical mixer (38), while the case of many photons in two modes has been analyzed in ref. 39, implying a possible application of the quantum Kravchuk–Fourier transform (40). We anticipate that most of these ideas could extend to interferences in an active optical medium.
Classical Baseline.
The two-photon quantum interference effect in amplification cannot be interpreted within a classical model of PDC, where a pair can be annihilated or created with some probability. We have two possible indistinguishable paths (the photon pair either going through the crystal or being replaced by another one) with equal individual probabilities but opposite probability amplitudes; hence, the resulting probability vanishes (whereas the two probabilities would add for classical particles). In order to assess an experimental verification of this effect, it is necessary to establish a classical baseline, namely to determine the depletion of the probability of coincident detections that can be interpreted classically. As a guide, consider first a classical model of the HOM effect where the two input photons are distinguishable. We have to add the double-transmission probability
Acknowledgements
We thank Ulrik L. Andersen, Maria V. Chekhova, Claude Fabre, Virginia D’Auria, Linran Fan, Radim Filip, Saikat Guha, Dmitri Horoshko, Mikhail I. Kolobov, Julien Laurat, Klaus Mölmer, Romain Mueller, Ognyan Oreshkov, Olivier Pfister, Wolfgang P. Schleich, and Sébastien Tanzilli as well as an anonymous referee for useful comments. M.G.J. acknowledges support from the Wiener-Anspach Foundation. This work was supported by the Fonds de la Recherche Scientifique - FNRS under grant PDR T.0224.18.
Data Availability.
There are no data underlying this work.
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Two-boson quantum interference in time
