Topological insulators combine insulating properties in the bulk with scattering-free transport along edges, supporting dissipationless unidirectional energy and information flow even in the presence of defects and disorder. The feasibility of engineering quantum Hamiltonians with photonic tools, combined with the availability of entangled photons, raises the intriguing possibility of employing topologically protected entangled states in optical quantum computing and information processing. However, while two-photon states built as a product of two topologically protected single-photon states inherit full protection from their single-photon “parents”, a high degree of non-separability may lead to rapid deterioration of the two-photon states after propagation through disorder. In this work, we identify physical mechanisms which contribute to the vulnerability of entangled states in topological photonic lattices. Further, we show that in order to maximize entanglement without sacrificing topological protection, the joint spectral correlation map of two-photon states must fit inside a well-defined topological window of protection.
Topological protection of entangled states is a promising avenue for photonic quantum technologies. Here, Tschernig et al. theoretically analyse the impact of disorder on topological protection of entangled two-photon states in periodic and aperiodic topological insulator lattices.
The prospect of generating topologically protected entangled states of several photons is a highly intriguing proposition1–3. Specifically, topological protection can enable robust transport of quantum information across disordered photonic structures without degradation4,5, just as efficiently as for single-particle wavepackets6–10.
In recent years, we have witnessed several experimental demonstrations of topological protection at the single-photon level in integrated one-dimensional lattice systems. Notably, Wang and co-workers11 showed that the fundamental quantum features of spatially entangled biphoton-states can be protected against disorder in the so-called Su-Schrieffer-Heeger (SSH) topological lattice. Interestingly, SSH lattices turned out to be equally effective in protecting polarization-entangled photon pairs12. Another important ingredient was provided by Tambasco et al.13 showing that Hong-Ou-Mandel two-photon interference of topological edge–modes is feasible, by implementing a topological beamsplitter in a judiciously engineered time-dependent Harper-model.
Concurrently, on the theory front several ideas have been suggested to investigate topological two-photon effects in linear14,15 and nonlinear16 lattice systems. In this regard, an intriguing proposition was recently put forward17, where the Bose-Hubbard model, which is topologically trivial for single particles, becomes topologically nontrivial for two interacting photons. That is, particle interactions have a dramatic impact on topological properties, not only modifying the topology of the spectra but also creating a topological order in otherwise topologically trivial systems.
In order to maximize the potential of topological photonic networks for transferring quantum information, it is indispensable to have a considerable number of edge modes at our disposal. One possibility is to use two-dimensional topological systems, which intrinsically support a multitude of topological edge-states18–20.
In two-dimensional photonic topologial insulators, single-particle edge-states reside in the gap existing between the energy bands supporting the bulk states21–23. Thus, breaking the topological protection requires disorder with sufficient strength to close the bandgap. For states describing two indistinguishable photons, the same bandgap is fundamentally lacking. The reason is because the propagation eigenvalues for two-photon eigenstates in a photonic system are given by the sum of the eigenvalues λ1, λ2 corresponding to the constituent individual photons,
In solids, the degeneracies described above lead to the decay of two-electron edge states when electron–electron correlations are substantial24–26. This decay mechanism is reminiscent of auto-ionization, where electron–electron correlations lead to energy exchange between the two particles, coupling two bound electronic excitations to an energy-degenerate bound-continuum two-electron state27,28.
Still, photonic systems are fundamentally different from solids, as the two photons do not readily interact with each other29. Consequently, the evolution operator for two-photon states, U(2)(z), breaks down into the product of two propagators for individual single-photon states, U(2)(z) = U(z) ⊗ U(z)30. Thus, a natural question to ask is whether such a factorization and the absence of bangap will prevent decoherence and dissipation of non-factorizable two-photon edge-states into the bulk?
In this work, we analyze possible mechanisms of dissipation of two-photon edge states into the bulk of two different topological insulator system, the Haldane lattice model and an aperiodic lattice corresponding to the quantum Hall effect. Our results show that the key to topological protection is to minimize the disorder-induced overlap of the initial two-photon (joint) spectrum with the edge–bulk and bulk–bulk spectral regions.
In lattice systems, static disorder can be introduced in either the site energies—termed diagonal disorder31—or in the coupling coefficients—so-called off-diagonal disorder32. In either case, static disorder is represented by a single-particle operator
To see this, we examine the second-order transition matrix elements between an initial two-photon edge–edge state


In contrast to dissipation, the situation with dephasing can be different: while each constituent state in an entangled superposition can be protected against disorder1, the overall superposition is, in general, not. To be precise, motion through different disordered regions may lead to disorder-induced random phase shifts between the states destroying the entanglement. To avoid this fate, all states in the superposition must travel across the same spatial region of the photonic structure, such that they are affected by disorder in the exact same manner33. These effects have been explored for spatial path-entangled states1, and for states built from an entangled superposition of an initial non-stationary state
A more appealing type of highly entangled two-photon states are multimode optical Gaussian states in which both photons are most likely to be found inhabiting any waveguide, within an excitation window, simultaneously36. The importance of such states is based on the fact that any phase difference arising among the paths becomes enhanced by a factor of two in comparison with single photon states37. Naturally, the enhanced phase sensitivity of such highly entangled two-photon states manifests as faster diffraction of the associated wavepackets propagating in any photonic system, periodic and disordered38. Therefore, it is not clear to what extent topological protection will persist for these types of highly entangled states.
In what follows we analyze the impact of disorder onto a continuum of two-photon states that extend from the correlated to the anti-correlated limits, passing through a completely separable state. For our analysis we consider two topological lattices, one periodic and one aperiodic. In the periodic case we consider the Haldane model39, and for the aperiodic we use a square lattice whose single-particle dynamics corresponds to the quantum Hall effect6,40 (information, S. Supporting material). The results for the Haldane model are presented here, while the quantum Hall effect lattice is discussed in the Supplementary Note 5.
In optics, a first-order approximation of the Haldane model can be implemented using a honeycomb lattice composed of helical waveguides as illustrated in Fig. 1a, see pioneering work41. In this system, every waveguide has a nearest-neighbor coupling κ1 and a complex second-nearest-neighbor coupling κ2 or



The Haldane photonic lattice.
a Photonic implementation of the Haldane system using a honeycomb lattice of helical waveguides. b Elementary hexagonal cell of the Haldane system, with real-valued nearest-neighbor coupling (blue arrows) κ1 = 1 and imaginary next-nearest-neighbor coupling (red arrows); κ2 = iκ1/5 along the arrow and − iκ1/5 in the opposite direction. c Pictorial view of the finite lattice used in our numerical analysis. d Single-photon spectrum formed by eigenvalues λn. In e and f we show the two-photon eigenspectra without and with disorder, respectively. Colors encode the two-photon eigenvalue
For pure states of two indistinguishable noninteracting particles the Hamiltonian is H2 = H ⊗ I + I ⊗ H, where H is the single-particle Hamiltonian and I is the identity operator42. The two-photon eigenstates are given by the symmetric tensor-product combinations of the single-photon eigenstates

In the absence of disorder, the eigenvalue spectrum for single-photon states in a finite lattice exhibits topological edge states in the bandgap43, Fig. 1d. In contrast, for two indistinguishable photons, the spectrum does not have a bandgap: the edge–edge states can have the same eigenvalues
To include disorder, we separate the lattice shown in Fig. 1c into three regions1. The left and right parts of the system are disorder-free, while its middle part exhibits diagonal disorder31, that is, random modifications of the on-site refractive index taken from a normal distribution with zero mean and variance σ = 1. Importantly, taking σ = 1 ensures that the disorder strength does not destroy the topological protection for single photons, since σ = 1 corresponds to half the size of the topological bandgap. The two-photon eigenspectrum in the presence of disorder is shown in Fig. 1f.
We now send trial two-photon wavepackets into the system. They are built from single-photon edge states and vary continuously from an unentangled product state, with Schmidt number SN = 1, to highly entangled two-photon states, SN ≫ 144,45, with the two photons either correlated or anti-correlated in space46.
To construct these states, we begin with protected single-photon states as a template,
Next, we construct our trial two-photon states as follows

Finally, we must ensure that the initial wavepackets only include edge states. To this end, we project our state onto the two-photon eigenstates



Initial two-photon states.
a, b, c Spatial correlation maps Pn,m over the 91 sites of the upper edge of the lattice. d, e, f Spectral correlation maps Sn,m in the
Figure 3a, b visualize this outcome by showing the single-photon spatial distribution and two-photon spectral correlation maps for the two-photon product state


Propagation of two-photon edge states.
a Probability density distribution for the reduced single-photon state and b the spectral correlation map for the product state
We now turn our attention to entangled two-photon states. Figure 3c, d depict R(n) and the spectral correlation maps for the two-photon state
To quantify the probability fraction of the states scattered into the bulk we compute the edge–mode content. For
We find that the conduit for dissipation of the two-photon edge–edge states is always provided by the edge–bulk states, which are degenerate in energy with the edge–edge states. Once disorder induces transitions into the edge–bulk states, they further transfer the amplitudes into the energy-degenerate bulk–bulk states, see Supplementary Movies M2 and M3. Hence, the key to topological protection is to minimize the disorder-induced overlap of the initial joint spectrum with the edge–bulk and bulk–bulk spectral regions, keeping it as close to the center as possible. That is, there is a topological protection window for two-photon states that offers the key guideline for designing robust two-photon states. To infer the protection window, we sent a probe product state with σc = σa = 0.01 through an ensemble of 1000 disordered lattices. This initial state is very well localized onto the edge region in real space, ensuring that all components within the state travel along very close paths. The spectral content of the state before and after the disorder is shown in in Fig. 4a, b. The components that have survived the impact of disorder are within the marked window—the topological window of protection. The joint spectral correlation map of any entangled state with varying σa and σc must fit inside this protection window to be robust against disorder.


Topological window of protection.
In order to identify the topological window of protection, we considered a spectrally broad product state with (σa = σc = 0.01) as initial state and propagate it through an ensemble of 1000 random Haldane lattices. In a we depict the spectral correlation map for the initial state. b depicts the ensemble-average of the spectral correlation maps inside the edge–edge subspace after the propagation through the ensemble of disordered lattices. We find that the only two-photon amplitudes that survive the disorder lie in the region indicated by the black square, which is the protection window. c shows the edge–mode content E and d the product of the edge–mode content and the Schmidt-number E ⋅ SN as a function of the parameters σa, σc of the initial states in the range σa, σc ∈ [0.01, 10].
In practice, to increase the amount of entanglement we need to increase σa
As evidence that our results are generic, in the sense that they apply to other two-dimensional topological systems, in the Supplementary Note 5 we have performed a similar analysis for an aperiodic topological lattice system6,40. We have found that the contour map of the edge-mode content E is not symmetric, implying that the correlated states are slightly less protected than their anti-correlated mirror-images. Nevertheless, we obtain the same qualitative features as in the Haldane model.
Before concluding, we would like to outline possible ways to generate the initial states and address the potential challenges for experimental observations of these effects. The initially highly correlated states can be implemented using standard spontaneous-parametric-down-conversion nonlinear crystals to generate photon pairs that are coupled to the edge of the lattice using a positive achromatic doublet lens as demonstrated in38. Anti-correlated photon pairs can be generated by applying the fractional Fourier transform to the highly correlated states49. The Haldane lattice has been previously demonstrated using femtosecond laser written waveguides as reported in41. Hence, the challenges are reduced to optimizing the fabrication for minimal scattering, absorption and bending losses associated with the helical waveguides.
These results lead to the following conclusions. Two issues have to be considered when constructing two-photon entangled edge states in topological systems: their dissipation into the bulk and the relative dephasing between the different components comprising the entangled state. Regarding dissipation, the two-photon edge states can be protected just as well as the single-photon edge states. Further, phase scrambling can also be minimized if the different components of the entangled state travel along the same path in the edge region. Both aims are achieved by keeping the spectral correlation map of the two-photon state in the center of the window of protection. Thus, attempts to increase entanglement must be balanced against keeping the spectral correlation maps of the two-photon states within the narrow spectral region at the very center of the single-photon gap—the topological window of protection. This limits the degree of entanglement one can safely encode in practice, but presents a clear strategy for creating useful states with high degree of entanglement and robustness.
Looking forward, one could take advantage of the static nature of disorder to circumvent entanglement-induced dissipation into the bulk. While the disorder-induced relative phase between the different product-state components of the entangled wavepacket may appear random due to the random nature of disorder, for static disorder scrambling and dissipation are nevertheless fixed. This opens an opportunity to find the windows of protection as we have done in the cases considered here, and generate robust wavepackets tailored to the particular disordered system at hand. From a practical perspective, the stability of entangled states up to relatively high Schmidt numbers offers practical guidelines for generating useful entangled edge states in topological photonic systems. Finally, our work may open the door to study topological protection of highly entangled multiphoton non-Gaussian states that fulfill the protection conditions.
The online version contains supplementary material available at 10.1038/s41467-021-22264-3.
We acknowledge support by the Open Access Publication Fund of Humboldt-Universität zu Berlin. K.T., A.P.L., and K.B. acknowledge support by the Deutsche Forschungsgemeinschaft (DFG) within the framework of the DFG priority program 1839 Tailored Disorder (BU 1107/ 12-2, PE 2602/2-2). A.J.-G. acknowledges funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement No 899794. M.I. acknowledges funding from the Deutsche Forschungsgemeinschaft under grant agreement IV 152/6-2. The work of DNC was partially supported by AFOSR (MURI FA9550-20-1-0322).
A.P.L., M.A.B., and D.N.C. initiated the project. A.P.L., M.A.B., D.N.C., M.I., and K.B. outlined the work. K.T., A.J.G., M.I., M.A.B., and A.P.L. developed the theory. K.T., K.B., and A.P.L. performed the simulations. All the authors discussed and analyzed the results. K.T., M.I., and A.P.L. wrote the manuscript with input from all coauthors. M.A.B. and A.P.L. coordinated the project.
Open Access funding enabled and organized by Projekt DEAL.
The data that support the findings of this study are available from the corresponding author upon reasonable request.
The Matlab programs used to simulate the systems discussed in the paper are available as supplementary software.
The authors declare no competing interests.
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